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| Title: | Dynamical theory of spectroscopy with femtosecond pulse excitation (III) - Transient rate equation in Liouville space | Authors: | Lu, J. Fan, K. Lee, S.-Y. |
Keywords: | Density matrix Femtosecond IBr Raman |
Issue Date: | Jun-1999 | Citation: | Lu, J.,Fan, K.,Lee, S.-Y. (1999-06). Dynamical theory of spectroscopy with femtosecond pulse excitation (III) - Transient rate equation in Liouville space. Science in China, Series A: Mathematics, Physics, Astronomy 42 (6) : 666-672. ScholarBank@NUS Repository. | Abstract: | A dynamical theory of spectroscopy with femtosecond pulse excitation is developed in Liouville space. By using density matrix formalism, the transient rate equation that can be reduced to the classical KHD expression in CW case is obtained. This theory is applied to the Raman excitation profile of IBr and the results are in agreement with the experiments. | Source Title: | Science in China, Series A: Mathematics, Physics, Astronomy | URI: | http://scholarbank.nus.edu.sg/handle/10635/76003 | ISSN: | 10069283 |
| Appears in Collections: | Staff Publications |
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