Please use this identifier to cite or link to this item: https://doi.org/10.1002/advs.201901129
Title: Atomic- and Molecular-Level Design of Functional Metal-Organic Frameworks (MOFs) and Derivatives for Energy and Environmental Applications
Authors: YILMAZ GAMZE 
PEH SHING BO 
Zhao Dan 
HO GHIM WEI 
Keywords: Science & Technology
Physical Sciences
Technology
Chemistry, Multidisciplinary
Nanoscience & Nanotechnology
Materials Science, Multidisciplinary
Chemistry
Science & Technology - Other Topics
Materials Science
atomic-molecular design
energy applications
environmental applications
metal-organic frameworks
reticular chemistry
OXYGEN REDUCTION REACTION
NITROGEN-DOPED GRAPHENE
HIGH-PERFORMANCE ELECTROCATALYSTS
ZEOLITIC-IMIDAZOLATE-FRAMEWORK
HYDROGEN EVOLUTION ACTIVITY
POROUS CARBON MATERIALS
PLATINUM SINGLE-ATOM
ACTIVE-SITES
HETEROGENEOUS CATALYSTS
COORDINATION POLYMER
Issue Date: 1-Sep-2019
Publisher: WILEY
Citation: YILMAZ GAMZE, PEH SHING BO, Zhao Dan, HO GHIM WEI (2019-09-01). Atomic- and Molecular-Level Design of Functional Metal-Organic Frameworks (MOFs) and Derivatives for Energy and Environmental Applications. ADVANCED SCIENCE 6 (21). ScholarBank@NUS Repository. https://doi.org/10.1002/advs.201901129
Abstract: © 2019 The Authors. Published by WILEY-VCH Verlag GmbH & Co. KGaA, Weinheim Continuing population growth and accelerated fossil-fuel consumption with recent technological advancements have engendered energy and environmental concerns, urging researchers to develop advanced functional materials to overcome the associated problems. Metal–organic frameworks (MOFs) have emerged as frontier materials due to their unique porous organic–inorganic hybrid periodic assembly and exceptional diversity in structural properties and chemical functionalities. In particular, the modular nature and modularity-dependent activity of MOFs and MOF derivatives have accentuated the delicate atomic- and molecular design and synthesis of MOFs, and their meticulous conversion into carbons and transition-metal-based materials. Synthetic control over framework architecture, content, and reactivity has led to unprecedented merits relevant to various energy and environmental applications. Herein, an overview of the atomic- and molecular-design strategies of MOFs to realize application-targeted properties is provided. Recent progress on the development of MOFs and MOF derivatives based on these strategies, along with their performance, is summarized with a special emphasis on design–structure and functionality–activity relationships. Next, the respective energy- and environmental-related applications of catalysis and energy storage, as well as gas storage-separation and water harvesting with close association to the energy–water–environment nexus are highlighted. Last, perspectives on current challenges and recommendations for further development of MOF-based materials are also discussed.
Source Title: ADVANCED SCIENCE
URI: https://scholarbank.nus.edu.sg/handle/10635/169559
ISSN: 2198-3844
DOI: 10.1002/advs.201901129
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