Please use this identifier to cite or link to this item:
|Title:||Composition-dependent ultra-high photoconductivity in ternary CdSxSe1-x nanobelts as measured by optical pump-terahertz probe spectroscopy|
|Keywords:||nanomaterials and nanostructures|
|Citation:||Liu, H., Lu, J., Zheng, M., Tang, S.H., Zhang, X., Sow, C.H. (2013-10). Composition-dependent ultra-high photoconductivity in ternary CdSxSe1-x nanobelts as measured by optical pump-terahertz probe spectroscopy. Nano Research 6 (11) : 808-821. ScholarBank@NUS Repository. https://doi.org/10.1007/s12274-013-0359-x|
|Abstract:||We employ optical pump-terahertz probe spectroscopy to investigate the composition-dependent photoconductivity in ternary CdSxSe1-x nanobelts. The observed carrier dynamics of CdS nanobelts display much shorter lifetime than those of ternary CdSxSe1-x nanobelts. This indicates the implementation of CdS nanobelts as ultrafast switching devices with a switching speed potentially up to 46.7 GHz. Surprisingly, ternary CdSxSe1-x nanobelts are found to exhibit much higher photoconductivity than binary CdS and CdSe. This is attributed to the higher photocarrier densities in ternary compounds. In addition, the presence of Se in samples resulted in prominent CdSe-like transverse optical (TO) phonon modes due to electron-phonon interactions. The strength of this mode shows a large drop upon photoexcitation but recovers gradually with time. These results demonstrated that growth of ternary nanostructures can be utilized to alleviate the high surface defect density in nanostructures and improve their photoconductivity. © 2013 Tsinghua University Press and Springer-Verlag Berlin Heidelberg.|
|Source Title:||Nano Research|
|Appears in Collections:||Staff Publications|
Show full item record
Files in This Item:
There are no files associated with this item.
checked on Sep 19, 2018
WEB OF SCIENCETM
checked on Sep 3, 2018
checked on Sep 21, 2018
Items in DSpace are protected by copyright, with all rights reserved, unless otherwise indicated.