Please use this identifier to cite or link to this item: https://doi.org/10.1016/j.watres.2014.02.030
Title: Performance of an optimized Zr-based nanoparticle-embedded PSF blend hollow fiber membrane in treatment of fluoride contaminated water
Authors: He, J.
Siah, T.-S.
Paul Chen, J. 
Keywords: Adsorption
Filtration
Fluoride
Hollow fiber membrane
Nano particle
Toxicity
XPS
Zirconium
Issue Date: 1-Jun-2014
Citation: He, J., Siah, T.-S., Paul Chen, J. (2014-06-01). Performance of an optimized Zr-based nanoparticle-embedded PSF blend hollow fiber membrane in treatment of fluoride contaminated water. Water Research 56 : 88-97. ScholarBank@NUS Repository. https://doi.org/10.1016/j.watres.2014.02.030
Abstract: Consumption of water that has excessive fluoride can cause adverse health impacts on human beings. A Zr-based nanoparticle-embedded PSF blend hollow fiber membrane was successfully prepared and optimized for removal of fluoride from the aqueous solution. Both static and dynamic adsorption of fluoride on the membrane was investigated. It was showed that the membrane could effectively remove fluoride within a wide pH ranging from 3 to 10. At neutral pH, the adsorption equilibrium was reached within 24h. The maximum adsorption capacity of the optimized membrane was 60.65mg/g, much higher than many commercial adsorbents. The presence of NO3-, SiO32- or HA has insignificant effects on the fluoride removal. However, the removal was retarded as the concentration of HCO3- or PO43- was increased. Furthermore, the membrane could remove fluoride efficiently through the continuous filtration, even in presence of natural organic matters. The spent membrane could be regenerated and then reused for the removal of fluoride with great efficiency. The adsorption history could be well described by an intraparticle diffusion model. The XPS analysis showed that the adsorption of fluoride was mainly associated with the ion-exchange between SO42- and F- ions. Finally, the toxicity analysis revealed that the treated water was safe for human consumption. © 2014 Elsevier Ltd.
Source Title: Water Research
URI: http://scholarbank.nus.edu.sg/handle/10635/91130
ISSN: 18792448
DOI: 10.1016/j.watres.2014.02.030
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