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https://doi.org/10.1063/1.4733982
Title: | Negative capacitance induced by redistribution of oxygen vacancies in the fatigued BiFeO 3-based thin film | Authors: | Ke, Q. Lou, X. Yang, H. Kumar, A. Zeng, K. Wang, J. |
Issue Date: | 9-Jul-2012 | Citation: | Ke, Q., Lou, X., Yang, H., Kumar, A., Zeng, K., Wang, J. (2012-07-09). Negative capacitance induced by redistribution of oxygen vacancies in the fatigued BiFeO 3-based thin film. Applied Physics Letters 101 (2) : -. ScholarBank@NUS Repository. https://doi.org/10.1063/1.4733982 | Abstract: | The capacitance dispersion in La and Mg co-substituted BiFeO 3 thin film has been studied at different stages of polarization switching. A negative capacitance (NC) behavior is observed in the sample that is fatigued above 10 9 switching cycles. The origin of the NC is investigated through analyzing relaxation processes and charge transport kinetics by admittance spectroscopy. An activation energy of ∼0.6 eV and a zero field mobility μ 0 5.33 ± 0.02 × 10 - 13 m 2 / Vs are thus obtained. A physical mechanism is proposed to explain this behavior. It involves a redistribution of oxygen vacancies, which are trapped at the film/electrode interface during the fatigue process. © 2012 American Institute of Physics. | Source Title: | Applied Physics Letters | URI: | http://scholarbank.nus.edu.sg/handle/10635/85478 | ISSN: | 00036951 | DOI: | 10.1063/1.4733982 |
Appears in Collections: | Staff Publications |
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