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|Title:||Enhanced tunability of the multiphoton absorption cross-section in seeded CdSe/CdS nanorod heterostructures||Authors:||Xing, G.
|Issue Date:||9-Aug-2010||Citation:||Xing, G., Chakrabortty, S., Chou, K.L., Mishra, N., Huan, C.H.A., Chan, Y., Sum, T.C. (2010-08-09). Enhanced tunability of the multiphoton absorption cross-section in seeded CdSe/CdS nanorod heterostructures. Applied Physics Letters 97 (6) : -. ScholarBank@NUS Repository. https://doi.org/10.1063/1.3479048||Abstract:||We present a method to separately tune the multiphoton absorption (MPA) and multiphoton excited photoluminescence using semiconductor core/enlarged-shell quantum dots (QDs), where the enlarged shell greatly enhances the MPA cross-sections while varying the core size facilitates emission wavelength selectivity. Following two-photon absorption (2PA) primarily in the shell and ultrafast charge-carrier localization to the core, luminescence occurs. We exemplify the validity of this method with CdSe/CdS nanorod heterostructures and find that the 2PA cross-section is enlarged to ∼1.4× 106 GM for 180 nm nanorods (with 800 nm, 150 fs laser pulse excitation) which is two to four orders larger than that of CdSe QDs. © 2010 American Institute of Physics.||Source Title:||Applied Physics Letters||URI:||http://scholarbank.nus.edu.sg/handle/10635/93758||ISSN:||00036951||DOI:||10.1063/1.3479048|
|Appears in Collections:||Staff Publications|
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