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|Title:||Superior performance asymmetric supercapacitors based on a directly grown commercial mass 3D Co3O4@Ni(OH)2 core-shell electrode||Authors:||Tang, C.-H.
|Issue Date:||13-Nov-2013||Citation:||Tang, C.-H., Yin, X., Gong, H. (2013-11-13). Superior performance asymmetric supercapacitors based on a directly grown commercial mass 3D Co3O4@Ni(OH)2 core-shell electrode. ACS Applied Materials and Interfaces 5 (21) : 10574-10582. ScholarBank@NUS Repository. https://doi.org/10.1021/am402436q||Abstract:||Pseudocapacitors based on fast surface Faradaic reactions can achieve high energy densities together with high power densities. Usually, researchers develop a thin layer of active materials to increase the energy density by enhancing the surface area; meanwhile, this sacrifices the mass loading. In this work, we developed a novel 3D core-shell Co3O4@Ni(OH) 2 electrode that can provide high energy density with very high mass loading. Core-shell porous nanowires (Co3O4@Ni(OH) 2) were directly grown on a Ni current collector as an integrated electrode/collector for the supercapacitor anode. This Co3O 4@Ni(OH)2 core-shell nanoarchitectured electrode exhibits an ultrahigh areal capacitance of 15.83 F cm-2. The asymmetric supercapacitor prototypes, assembled using Co3O4@Ni(OH) 2 as the anode, reduced graphene oxide (RGO) or active carbon (AC) as the cathode, and 6 M aqueous KOH as the electrolyte, exhibit very high energy densities falling into the energy-density range of Li-ion batteries. Because of the large mass loading and high energy density, the prototypes can drive a minifan or light a bulb even though the size is very small. These results indicate that our asymmetric supercapacitors have outstanding potential in commercial applications. Systematic study and scientific understanding were carried out. © 2013 American Chemical Society.||Source Title:||ACS Applied Materials and Interfaces||URI:||http://scholarbank.nus.edu.sg/handle/10635/86744||ISSN:||19448244||DOI:||10.1021/am402436q|
|Appears in Collections:||Staff Publications|
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