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|Title:||Structure and properties of hot-pressed lead-free (Ba0.85Ca 0.15)(Zr0.1Ti0.9)O3 piezoelectric ceramics||Authors:||Ye, S.
|Issue Date:||21-Nov-2013||Citation:||Ye, S., Fuh, J., Lu, L., Chang, Y.-L., Yang, J.-R. (2013-11-21). Structure and properties of hot-pressed lead-free (Ba0.85Ca 0.15)(Zr0.1Ti0.9)O3 piezoelectric ceramics. RSC Advances 3 (43) : 20693-20698. ScholarBank@NUS Repository. https://doi.org/10.1039/c3ra43429j||Abstract:||Randomly-oriented and textured (Ba0.85Ca0.15)(Zr 0.1Ti0.9)O3 (BCZT) ceramics are prepared by a hot-pressing (HP) method. The phase structure, microstructure, and electrical properties are systematically investigated. Structural analysis shows a decrease in tetragonality of the hot-pressed samples. The orientation of the as-processed ceramics is studied by X-ray diffraction and electron backscatter diffraction, revealing an increase in texture of the hot-pressed textured BCZT ceramics. Microstructure characterization demonstrates that the hot-pressing can greatly improve the densification of the BCZT ceramics. Dielectric constant measurement obeys a modified Curie-Weiss law. The relaxor-like behavior is decreased in hot-pressed samples. The Curie temperatures of the hot-pressed BCZT (BCZT-HP) and the hot-pressed BCZT with texture templates (BCZT-T-HP) ceramics are greatly increased to 76 °C and 90 °C, respectively. The optimum piezoelectric properties for the BCZT-HP and BCZT-T-HP ceramics are d 33 = 510 pC N-1, kp = 44%, d31 = -182 pC N-1, k31 = 23% and d33 = 580 pC N -1, kp = 49%, d31 = -204 pC N-1, k31 = 31%, respectively. Therefore, the BCZT-HP and BCZT-T-HP ceramics are promising lead-free piezoelectric ceramics which can be used in higher temperature than their counterparts prepared by conventional sintering. © The Royal Society of Chemistry 2013.||Source Title:||RSC Advances||URI:||http://scholarbank.nus.edu.sg/handle/10635/85677||ISSN:||20462069||DOI:||10.1039/c3ra43429j|
|Appears in Collections:||Staff Publications|
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