Please use this identifier to cite or link to this item: https://doi.org/10.1039/c9ta00942f
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dc.titleMaximizing the utility of single atom electrocatalysts on a 3D graphene nanomesh
dc.contributor.authorChi, Kai
dc.contributor.authorChen, Zhongxin
dc.contributor.authorXiao, Fei
dc.contributor.authorGuo, Wei
dc.contributor.authorXi, Wei
dc.contributor.authorLiu, Jing
dc.contributor.authorYan, Huan
dc.contributor.authorZhang, Zheye
dc.contributor.authorXiao, Jian
dc.contributor.authorLiu, Jia
dc.contributor.authorLuo, Jun
dc.contributor.authorWang, Shuai
dc.contributor.authorLoh, Kian Ping
dc.date.accessioned2020-07-21T03:27:51Z
dc.date.available2020-07-21T03:27:51Z
dc.date.issued2019-07-14
dc.identifier.citationChi, Kai, Chen, Zhongxin, Xiao, Fei, Guo, Wei, Xi, Wei, Liu, Jing, Yan, Huan, Zhang, Zheye, Xiao, Jian, Liu, Jia, Luo, Jun, Wang, Shuai, Loh, Kian Ping (2019-07-14). Maximizing the utility of single atom electrocatalysts on a 3D graphene nanomesh. JOURNAL OF MATERIALS CHEMISTRY A 7 (26) : 15575-15579. ScholarBank@NUS Repository. https://doi.org/10.1039/c9ta00942f
dc.identifier.issn20507488
dc.identifier.issn20507496
dc.identifier.urihttps://scholarbank.nus.edu.sg/handle/10635/171630
dc.description.abstract© 2019 The Royal Society of Chemistry. Single atom catalysis has recently become the most active frontier in heterogeneous catalysis, however, its performance is practically limited by the exposure of single atoms to reactants. Herein, we synthesized a vertically aligned N-doped graphene nanomesh array (VNGNMA) with a high density of in-plane surface holes and out-of-plane interconnected, vertically aligned structures to facilitate the diffusion of reactants and maximize the utility of single atoms in the liquid phase. Pd and Pt single atom catalysts supported on a 3D graphene nanomesh outperformed benchmark Pt/C and conventional single atom catalysts for the hydrogen evolution reaction due to rapid mass transport.
dc.language.isoen
dc.publisherRoyal Society of Chemistry
dc.sourceElements
dc.subjectScience & Technology
dc.subjectPhysical Sciences
dc.subjectTechnology
dc.subjectChemistry, Physical
dc.subjectEnergy & Fuels
dc.subjectMaterials Science, Multidisciplinary
dc.subjectChemistry
dc.subjectMaterials Science
dc.subjectELECTRON-MICROSCOPY
dc.subjectNANOPARTICLES
dc.subjectENERGY
dc.subjectCATALYSTS
dc.subjectEFFICIENT
dc.subjectSTRATEGIES
dc.subjectREDUCTION
dc.subjectDESIGN
dc.typeArticle
dc.date.updated2020-05-31T14:30:46Z
dc.contributor.departmentDEPT OF CHEMISTRY
dc.description.doi10.1039/c9ta00942f
dc.description.sourcetitleJOURNAL OF MATERIALS CHEMISTRY A
dc.description.volume7
dc.description.issue26
dc.description.page15575-15579
dc.published.statePublished
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