Please use this identifier to cite or link to this item:
|Title:||Ultrafast and nanoscale plasmonic phenomena in exfoliated graphene revealed by infrared pump-probe nanoscopy|
Castro Neto, A.H.
|Citation:||Wagner, M., Fei, Z., McLeod, A.S., Rodin, A.S., Bao, W., Iwinski, E.G., Zhao, Z., Goldflam, M., Liu, M., Dominguez, G., Thiemens, M., Fogler, M.M., Castro Neto, A.H., Lau, C.N., Amarie, S., Keilmann, F., Basov, D.N. (2014-02-12). Ultrafast and nanoscale plasmonic phenomena in exfoliated graphene revealed by infrared pump-probe nanoscopy. Nano Letters 14 (2) : 894-900. ScholarBank@NUS Repository. https://doi.org/10.1021/nl4042577|
|Abstract:||Pump-probe spectroscopy is central for exploring ultrafast dynamics of fundamental excitations, collective modes, and energy transfer processes. Typically carried out using conventional diffraction-limited optics, pump-probe experiments inherently average over local chemical, compositional, and electronic inhomogeneities. Here, we circumvent this deficiency and introduce pump-probe infrared spectroscopy with ∼20 nm spatial resolution, far below the diffraction limit, which is accomplished using a scattering scanning near-field optical microscope (s-SNOM). This technique allows us to investigate exfoliated graphene single-layers on SiO2 at technologically significant mid-infrared (MIR) frequencies where the local optical conductivity becomes experimentally accessible through the excitation of surface plasmons via the s-SNOM tip. Optical pumping at near-infrared (NIR) frequencies prompts distinct changes in the plasmonic behavior on 200 fs time scales. The origin of the pump-induced, enhanced plasmonic response is identified as an increase in the effective electron temperature up to several thousand Kelvin, as deduced directly from the Drude weight associated with the plasmonic resonances. © 2014 American Chemical Society.|
|Source Title:||Nano Letters|
|Appears in Collections:||Staff Publications|
Show full item record
Files in This Item:
There are no files associated with this item.
checked on Jul 16, 2018
WEB OF SCIENCETM
checked on Jun 20, 2018
checked on Jun 1, 2018
Items in DSpace are protected by copyright, with all rights reserved, unless otherwise indicated.